I've been obsessed with acrylic paint pens lately...I've discovered Montana and Liquitex artists' paint pens, and have been using them for everything I can think of in a painting: line, of course, to accent or create focal points, and misty smudges to create an atmosphere or lay a bit of a pale background for some later washes, drips of acrylic ink, or strokes with watercolor brush pens.
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